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Verfasst von:Legrand, Michel [VerfasserIn]   i
 Preunkert, Susanne [VerfasserIn]   i
 Weller, Rolf [VerfasserIn]   i
 Zipf, Lars [VerfasserIn]   i
 Elsässer, Christoph [VerfasserIn]   i
 Merchel, Silke [VerfasserIn]   i
 Rugel, Georg [VerfasserIn]   i
 Wagenbach, Dietmar [VerfasserIn]   i
Titel:Year-round record of bulk and size-segregated aerosol composition in central Antarctica (Concordia site) - Part 2
Titelzusatz:biogenic sulfur (sulfate and methanesulfonate) aerosol
Verf.angabe:Michel Legrand, Susanne Preunkert, Rolf Weller, Lars Zipf, Christoph Elsässer, Silke Merchel, Georg Rugel, Dietmar Wagenbach
E-Jahr:2017
Jahr:24 November 2017
Umfang:19 S.
Fussnoten:Gesehen am 09.04.2020
Titel Quelle:Enthalten in: Atmospheric chemistry and physics
Ort Quelle:Katlenburg-Lindau : EGU, 2001
Jahr Quelle:2017
Band/Heft Quelle:17(2017), 22, Seite 14055-14073
ISSN Quelle:1680-7324
Abstract:Multiple year-round (2006–2015) records of the bulk and size-segregated composition of aerosol were obtained at the inland site of Concordia located in East Antarctica. The well-marked maximum of non-sea-salt sulfate (nssSO4) in January (100±28ngm−3 versus 4.4±2.3ngm−3 in July) is consistent with observations made at the coast (280±78ngm−3 in January versus 16±9ngm−3 in July at Dumont d'Urville, for instance). In contrast, the well-marked maximum of MSA at the coast in January (60±23ngm−3 at Dumont d'Urville) is not observed at Concordia (5.2±2.0ngm−3 in January). Instead, the MSA level at Concordia peaks in October (5.6±1.9ngm−3) and March (14.9±5.7ngm−3). As a result, a surprisingly low MSA-to-nssSO4 ratio (RMSA) is observed at Concordia in mid-summer (0.05±0.02 in January versus 0.25±0.09 in March). We find that the low value of RMSA in mid-summer at Concordia is mainly driven by a drop of MSA levels that takes place in submicron aerosol (0.3µm diameter). The drop of MSA coincides with periods of high photochemical activity as indicated by high ozone levels, strongly suggesting the occurrence of an efficient chemical destruction of MSA over the Antarctic plateau in mid-summer. The relationship between MSA and nssSO4 levels is examined separately for each season and indicates that concentration of non-biogenic sulfate over the Antarctic plateau does not exceed 1ngm−3 in fall and winter and remains close to 5ngm−3 in spring. This weak non-biogenic sulfate level is discussed in the light of radionuclides (210Pb, 10Be, and 7Be) also measured on bulk aerosol samples collected at Concordia. The findings highlight the complexity in using MSA in deep ice cores extracted from inland Antarctica as a proxy of past dimethyl sulfide emissions from the Southern Ocean.
DOI:doi:10.5194/acp-17-14055-2017
URL:Bitte beachten Sie: Dies ist ein Bibliographieeintrag. Ein Volltextzugriff für Mitglieder der Universität besteht hier nur, falls für die entsprechende Zeitschrift/den entsprechenden Sammelband ein Abonnement besteht oder es sich um einen OpenAccess-Titel handelt.

Volltext: https://doi.org/https://doi.org/10.5194/acp-17-14055-2017
 Volltext: https://www.atmos-chem-phys.net/17/14055/2017/
 DOI: https://doi.org/10.5194/acp-17-14055-2017
Datenträger:Online-Ressource
Sprache:eng
K10plus-PPN:1694337812
Verknüpfungen:→ Zeitschrift

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