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Verfasst von:Kaldun, Andreas [VerfasserIn]   i
 Blättermann, Alexander [VerfasserIn]   i
 Stooß, Veit [VerfasserIn]   i
 Donsa, S. [VerfasserIn]   i
 Wei, H. [VerfasserIn]   i
 Pazourek, R. [VerfasserIn]   i
 Nagele, S. [VerfasserIn]   i
 Ott, Christian [VerfasserIn]   i
 Lin, C. D. [VerfasserIn]   i
 Burgdörfer, J. [VerfasserIn]   i
 Pfeifer, Thomas [VerfasserIn]   i
Titel:Observing the ultrafast buildup of a Fano resonance in the time domain
Verf.angabe:A. Kaldun, A. Blättermann, V. Stooß, S. Donsa, H. Wei, R. Pazourek, S. Nagele, C. Ott, C. D. Lin, J. Burgdörfer, T. Pfeifer
E-Jahr:2016
Jahr:[2016]
Umfang:4 S.
Illustrationen:Diagramme
Teil:volume:354
 year:2016
 number:6313
 pages:738-741
 extent:4
Fussnoten:Gesehen am 07.05.2020
Titel Quelle:Enthalten in: Science
Ort Quelle:Washington, DC [u.a.] : American Association for the Advancement of Science, 1880
Jahr Quelle:2016
Band/Heft Quelle:354(2016), 6313, Seite 738-741
ISSN Quelle:1095-9203
Abstract:Watching as helium goes topsy-turvy - Theorists have long pondered the underpinnings of the Fano resonance, a spectral feature that resembles adjacent rightside-up and upside-down peaks. An especially well-studied instance of this feature appears in the electronic spectrum of helium as a transient state undergoes delayed ionization. Two studies have now traced the dynamics of this state in real time. Gruson et al. used photoelectron spectroscopy to extract the amplitude and phase of the electron wave packet after inducing its interference with reference wave packets tuned into resonance at variable delays. Kaldun et al. used extreme ultraviolet absorption spectroscopy to probe the transient state while variably forcing ionization with a strong near-infrared field. - Science, this issue pp. 734 and 738 - Although the time-dependent buildup of asymmetric Fano line shapes in absorption spectra has been of great theoretical interest in the past decade, experimental verification of the predictions has been elusive. Here, we report the experimental observation of the emergence of a Fano resonance in the prototype system of helium by interrupting the autoionization process of a correlated two-electron excited state with a strong laser field. The tunable temporal gate between excitation and termination of the resonance allows us to follow the formation of a Fano line shape in time. The agreement with ab initio calculations validates our experimental time-gating technique for addressing an even broader range of topics, such as the emergence of electron correlation, the onset of electron-internuclear coupling, and quasi-particle formation. - Ultrafast spectroscopy traces the dynamics of a transient excited state in helium underlying appearance of a Fano resonance. - Ultrafast spectroscopy traces the dynamics of a transient excited state in helium underlying appearance of a Fano resonance.
DOI:doi:10.1126/science.aah6972
URL:Bitte beachten Sie: Dies ist ein Bibliographieeintrag. Ein Volltextzugriff für Mitglieder der Universität besteht hier nur, falls für die entsprechende Zeitschrift/den entsprechenden Sammelband ein Abonnement besteht oder es sich um einen OpenAccess-Titel handelt.

Volltext ; Verlag: https://doi.org/10.1126/science.aah6972
 Volltext: https://science.sciencemag.org/content/354/6313/738
 DOI: https://doi.org/10.1126/science.aah6972
Datenträger:Online-Ressource
Sprache:eng
K10plus-PPN:1697643434
Verknüpfungen:→ Zeitschrift

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