| |  Online-Ressource |
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| Verfasst von: | Ding, Thomas [VerfasserIn]  |
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| | Ott, Christian [VerfasserIn] |
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| | Kaldun, Andreas [VerfasserIn] |
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| | Blättermann, Alexander [VerfasserIn] |
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| | Meyer, Kristina [VerfasserIn] |
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| | Stooß, Veit [VerfasserIn] |
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| | Rebholz, Marc [VerfasserIn] |
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| | Birk, Paul [VerfasserIn] |
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| | Hartmann, Maximilian [VerfasserIn] |
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| | Brown, Andrew [VerfasserIn] |
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| | Hart, Hugo Van Der [VerfasserIn] |
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| | Pfeifer, Thomas [VerfasserIn] |
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| Titel: | Time-resolved four-wave-mixing spectroscopy for inner-valence transitions |
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| Verf.angabe: | Thomas Ding, Christian Ott, Andreas Kaldun, Alexander Blättermann, Kristina Meyer, Veit Stooss, Marc Rebholz, Paul Birk, Maximilian Hartmann, Andrew Brown, Hugo Van Der Hart, and Thomas Pfeifer |
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| E-Jahr: | 2016 |
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| Jahr: | 5 January 2016 |
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| Umfang: | 4 S. |
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| Teil: | volume:41 |
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| | year:2016 |
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| | number:4 |
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| | pages:709-712 |
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| | extent:4 |
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| Fussnoten: | Gesehen am 08.05.2020 |
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| Titel Quelle: | Enthalten in: Optics letters |
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| Ort Quelle: | Washington, DC : Soc., 1977 |
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| Jahr Quelle: | 2016 |
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| Band/Heft Quelle: | 41(2016), 4, Seite 709-712 |
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| ISSN Quelle: | 1539-4794 |
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| Abstract: | Noncollinear four-wave-mixing (FWM) techniques at near-infrared (NIR), visible, and ultraviolet frequencies have been widely used to map vibrational and electronic couplings, typically in complex molecules. However, correlations between spatially localized inner-valence transitions among different sites of a molecule in the extreme ultraviolet (XUV) spectral range have not been observed yet. As an experimental step toward this goal, we perform time-resolved FWM spectroscopy with femtosecond NIR and attosecond XUV pulses. The first two pulses (XUV-NIR) coincide in time and act as coherent excitation fields, while the third pulse (NIR) acts as a probe. As a first application, we show how coupling dynamics between odd- and even-parity, inner-valence excited states of neon can be revealed using a two-dimensional spectral representation. Experimentally obtained results are found to be in good agreement with ab initio time-dependent R-matrix calculations providing the full description of multielectron interactions, as well as few-level model simulations. Future applications of this method also include site-specific probing of electronic processes in molecules. |
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| DOI: | doi:10.1364/OL.41.000709 |
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| URL: | Bitte beachten Sie: Dies ist ein Bibliographieeintrag. Ein Volltextzugriff für Mitglieder der Universität besteht hier nur, falls für die entsprechende Zeitschrift/den entsprechenden Sammelband ein Abonnement besteht oder es sich um einen OpenAccess-Titel handelt.
Volltext ; Verlag: https://doi.org/10.1364/OL.41.000709 |
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| | Volltext: https://www.osapublishing.org/ol/abstract.cfm?uri=ol-41-4-709 |
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| | DOI: https://doi.org/10.1364/OL.41.000709 |
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| Datenträger: | Online-Ressource |
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| Sprache: | eng |
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| Sach-SW: | Absorption spectroscopy |
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| | Attosecond pulses |
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| | Electric fields |
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| | Molecules |
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| | Near infrared radiation |
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| | Photoelectron spectroscopy |
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| K10plus-PPN: | 1697750273 |
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| Verknüpfungen: | → Zeitschrift |
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Time-resolved four-wave-mixing spectroscopy for inner-valence transitions / Ding, Thomas [VerfasserIn]; 5 January 2016 (Online-Ressource)
