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Verfasst von:Schubert, Ina [VerfasserIn]   i
 Huck, Christian [VerfasserIn]   i
 Kröber, Philipp [VerfasserIn]   i
 Neubrech, Frank [VerfasserIn]   i
 Pucci, Annemarie [VerfasserIn]   i
 Toimil-Molares, Maria Eugenia [VerfasserIn]   i
 Trautmann, Christina [VerfasserIn]   i
 Vogt, Jochen [VerfasserIn]   i
Titel:Porous gold nanowires
Titelzusatz:plasmonic response and surface-enhanced infrared absorption
Verf.angabe:Ina Schubert, Christian Huck, Philipp Kröber, Frank Neubrech, Annemarie Pucci, Maria Eugenia Toimil‐Molares, Christina Trautmann, and Jochen Vogt
E-Jahr:2016
Jahr:August 9, 2016
Umfang:8 S.
Fussnoten:Gesehen am 22.05.2020
Titel Quelle:Enthalten in: Advanced optical materials
Ort Quelle:Weinheim : Wiley-VCH, 2013
Jahr Quelle:2016
Band/Heft Quelle:4(2016), 11, Seite 1838-1845
ISSN Quelle:2195-1071
Abstract:Because of its extended surface area porous gold is of potential interest for surface-enhanced spectroscopy methods. Optical properties of porous and smooth gold nanowires of similar diameter are analyzed with infrared spectroscopy and modeled with finite-difference time-domain simulations. By electrochemical deposition in ion-track etched polymer smooth gold and gold-silver alloy nanowires are synthesized. Porous gold nanowires are subsequently obtained by dealloying. The porosity clearly affects important plasmonic characteristics, resulting in a strong redshift of the resonant wavelength, and significant line broadening, which can be convincingly explained by effective Drude parameters related to a lowered average electron density and a higher electron scattering in the porous gold, respectively. Finally, the sensing performance of porous wires is tested by surface-enhanced infrared absorption. The measurements show a similar vibrational signal contrast for smooth and porous wires. This is explained by simulations which reveal that the nanowire near-field modeled with bulk gold data is higher and thus accordingly the vibrational signal is enhanced compared to nanowires modeled with the effective Drude parameters of porous gold. This means that the advantages offered by the larger surface of porous wires are counterbalanced by lower near-field strength.
DOI:doi:10.1002/adom.201600430
URL:Bitte beachten Sie: Dies ist ein Bibliographieeintrag. Ein Volltextzugriff für Mitglieder der Universität besteht hier nur, falls für die entsprechende Zeitschrift/den entsprechenden Sammelband ein Abonnement besteht oder es sich um einen OpenAccess-Titel handelt.

Volltext: https://doi.org/10.1002/adom.201600430
 Volltext: https://onlinelibrary.wiley.com/doi/abs/10.1002/adom.201600430
 DOI: https://doi.org/10.1002/adom.201600430
Datenträger:Online-Ressource
Sprache:eng
Sach-SW:gold nanoantennas
 infrared spectroscopy
 localized surface plasmons
 porous gold antennas
 SEIRA
K10plus-PPN:1698694601
Verknüpfungen:→ Zeitschrift

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