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Verfasst von:Bâldea, Ioan [VerfasserIn]   i
 Xie, Zuoti [VerfasserIn]   i
 Frisbie, C. Daniel [VerfasserIn]   i
Titel:Uncovering a law of corresponding states for electron tunneling in molecular junctions
Verf.angabe:Ioan Bâldea, Zuoti Xie and C. Daniel Frisbie
E-Jahr:2015
Jahr:18 May 2015
Umfang:7 S.
Fussnoten:Gesehen am 29.07.2020
Titel Quelle:Enthalten in: Nanoscale
Ort Quelle:Cambridge : RSC Publ., 2009
Jahr Quelle:2015
Band/Heft Quelle:7(2015), 23, Seite 10465-10471
ISSN Quelle:2040-3372
Abstract:Laws of corresponding states known so far demonstrate that certain macroscopic systems can be described in a universal manner in terms of reduced quantities, which eliminate specific substance properties. To quantitatively describe real systems, all these laws of corresponding states contain numerical factors adjusted empirically. Here, we report a law of corresponding states deduced analytically for charge transport via tunneling in molecular junctions, which we validate against current-voltage measurements for conducting probe atomic force microscope junctions based on benchmark molecular series (oligophenylenedithiols and alkanedithiols) and electrodes (silver, gold, and platinum), as well as against transport data for scanning tunneling microscope junctions. Two salient features distinguish the present law of corresponding states from all those known previously. First, it is expressed by a universal curve free of empirical parameters. Second, it demonstrates that a universal behavior is not necessarily affected by strong stochastic fluctuations often observed in molecular electronics. An important and encouraging message of this finding is that transport behavior across different molecular platforms can be similar and extraordinarily reproducible.
DOI:doi:10.1039/C5NR02225H
URL:Bitte beachten Sie: Dies ist ein Bibliographieeintrag. Ein Volltextzugriff für Mitglieder der Universität besteht hier nur, falls für die entsprechende Zeitschrift/den entsprechenden Sammelband ein Abonnement besteht oder es sich um einen OpenAccess-Titel handelt.

Volltext ; Verlag: https://doi.org/10.1039/C5NR02225H
 Volltext: https://pubs.rsc.org/en/content/articlelanding/2015/nr/c5nr02225h
 DOI: https://doi.org/10.1039/C5NR02225H
Datenträger:Online-Ressource
Sprache:eng
K10plus-PPN:1725843994
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