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Verfasst von:Cederbaum, Lorenz S. [VerfasserIn]   i
 Kuleff, Alexander I. [VerfasserIn]   i
Titel:Impact of cavity on interatomic Coulombic decay
Verf.angabe:Lorenz S. Cederbaum, Alexander I. Kuleff
E-Jahr:2021
Jahr:02 July 2021
Umfang:8 S.
Fussnoten:Gesehen am 04.08.2021
Titel Quelle:Enthalten in: Nature Communications
Ort Quelle:[London] : Nature Publishing Group UK, 2010
Jahr Quelle:2021
Band/Heft Quelle:12(2021), Artikel-ID 4083, Seite 1-8
ISSN Quelle:2041-1723
Abstract:The interatomic Coulombic decay (ICD) is an efficient electronic decay process of systems embedded in environment. In ICD, the excess energy of an excited atom A is efficiently utilized to ionize a neighboring atom B. In quantum light, an ensemble of atoms A form polaritonic states which can undergo ICD with B. Here we investigate the impact of quantum light on ICD and show that this process is strongly altered compared to classical ICD. The ICD rate depends sensitively on the atomic distribution and orientation of the ensemble. It is stressed that in contrast to superposition states formed by a laser, forming polaritons by a cavity enables to control the emergence and suppression, as well as the efficiency of ICD. Interatomic Coulombic decay, ICD, is commonly observed in systems weakly bound to different environments. Here the authors discuss the ICD in an electromagnetic cavity and show that the entanglement of atoms can change ICD rates substantially and be used to control the ICD process.
DOI:doi:10.1038/s41467-021-24221-6
URL:kostenfrei: Volltext: https://doi.org/10.1038/s41467-021-24221-6
 kostenfrei: Volltext: https://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcAuth=DynamicDOIArticle&SrcApp=WOS&KeyAID=10.1038%2 ...
 DOI: https://doi.org/10.1038/s41467-021-24221-6
Datenträger:Online-Ressource
Sprache:eng
Sach-SW:auger
 chemistry
 dynamics
 electrons
 energy-transfer
 vibrational-energy
K10plus-PPN:1765445507
Verknüpfungen:→ Zeitschrift
 
 
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